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Stereo-divergent atom transfer radical cyclization of engineered cytochrome P450

 Last Update: 2022-01-10
 Source: Internet
 Author: User

Free radical cyclization is easy

Metallic enzymes contain metal cofactors and can sometimes be used to catalyze reactions different from their natural functions

Drawing inspiration from heme-based free radical polymerization, ZhouWait.

Due to the lack of exploitable stereo-controlling elements in the synthesis system, it is notoriously difficult to control the absolute and relative stereochemistry of the free radical process in asymmetric catalysis

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