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Combinatorial methods have been applied with a measure of success in the field of metal ion coordination chemistry (
1
–
5
). High-throughput screening methods have been used to facilitate the discovery of new catalysts and to design ligands for binding metal ions (
6
–
9
). Metal ion coordination complexes have been central to the development of dynamic combinatorial methods as well. Dynamic combinatorial methods utilize a library whose composition is con-trolled through reversible interactions with a target molecule (
10
,
11
). Metalligand bonds are often labile enough to undergo reversible bond formation under mild conditions, making metal ions ideal components for dynamic librar-ies. Such metal ion complexes are used in dynamic combinatorial libraries for the purpose of designing compounds with unusual shapes or recognition properties (
12
,
13
).
